How to handle the content of a Dictionary to store it in an array

Hello to all,

Please some help here.

I have and dictionary of 2 dimensions. The code is like below:

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I'd like to manipulate the content of the Dic1 in order to get an array like shown below.
How can I do this?

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I've been trying to assing the values of Dic1 like below, but I'm only able to assign in a single command
the keys and the items x,y,z but not the content of the items (the numbers).

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Thanks for any help.