the only way i could think of coming close to this is to utilize a helper column in column B. This will count the amount of time above the # has occured. It will return ERROR in the cell next to column A where the count has gotten to high. Mind you they can still input a 2,3, or 4 in column A but will keep saying ERROR in column B.
See my attached workbook.
Dropdown lists are in A1:A20
Helper formula is in B1:B20.
Formula:
=IFERROR(CHOOSE($A1,,IF(COUNTIF($A$1:$A1,$A1)>2,"ERROR",""),IF(COUNTIF($A$1:$A1,$A1)>3,"ERROR",""),IF(COUNTIF($A$1:$A1,$A1)>4,"ERROR","")),"")
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